The CIS-Lamda guys may be able to use MegaSquirt to control the frequency valve. Remember that the WUR is just a fuel pressure regulator.
http://unwiredtools.com/utcis.asp
To me it looks like an adjustable fuel pressure regulator with a stepper motor.
For A1 and A2 chassis cars:
CIS-Basic 1976.5-1983 (e.g., Rabbit pick-up)
CIS-Lambda 1980.5-1989 (e.g., Rabbit GTI, Golf GL)
CIE-E 1984.5-1989 (e.g., GTI 8V, GLI 1.8L 16V)
CIS-Motronic 1989.5-1992 (e.g., GLI 2L 16V)
Digifant (all types) 1987.5-1992 (e.g., Calif. Golf, Rabbit Cabriolet)
I agree that a MegaSquirt or like system could dynamically adjust mixture on CIS-Lambda by controlling the frequency valve. But, there is a question in my mind about the delayed effect at the injectors. While it might be fast enough to make a difference on a long straight, for example, it seems like it might actually make matters worse in dynamic transitions (unless one were to re-write MegaSquirt as an adaptive control system, probably with learned control parameters for each driver and possibly for each track).
A better choice, if available on the IT model line, would be to control the CIS-E/CIS-Motronic fuel distributor's differential pressure valve, which is faster acting, more accurate, and has a finer control input. With my unfinished ITA Scirocco 16V build, I had hoped to use MegaSquirt&Spark with CIS-E (since I don't think the 16V ever came with Digifant).
Edit: For those unsure if the particular car ever came with CIS-E (or CIS-Lambda, for that matter), don't just assume that it didn't. Check for late-production California cars, Wolfsburg Editions, and possible mid-year switch-overs, especially in the final year of production.